The treble of the LCD-2.1 is indeed shelved down compared to many headphones, but the Siemens CCa in the Lyr add strong, tight bass, tremendous energy with the drums, larger soundstage, more air, and a very nice treble extension and details. They're not easy to find, and not cheap, but if you want to know how good your Lyr/LCD-2.1 combo can sound, they're a good starting point.
If you want to bring out the most of your LCD-2's treble, I also suggest you try other cables. Though I sold my LCD-2.1 before receiving the Q cables, they really improve my LCD-3's treble, much more than I expected, without any penalty to the bass (it's in fact tighter with the Qs). Since Both headphones share the same overall sound signature, I suppose they would do the same to the LCD-2.1.