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For me the music comes first and I really enjoy headphones that get out of the way of the music, and I really enjoy music more when I get out of the way of the headphones. I find that both the HD 650 and LCD-2 get out of the recording's way, but the LCD-2 just seems to reveal extra details that seem make the experience more intriguing.
Re. what you said about a source and amp, I'm currently using the LCD-2 with a Lavry DA 10, which from what I've read I seem to have a fairly accurate source, and for me music is sounding really enjoyable with that and the LCD-2. What kind of differences do you reckon upgrading the amp (and possibly source) would bring in relation to an iTunes-Lavry-headphone rig?
You've described my main dynamic rig pretty well here (though I've added a quite coloured tube amp recently for something different). I used to own a DA 10, but didn't feel it was great with those hard-to-get-sounding-real instruments such as pianos and violins. Maybe if I had been using better than just an optical connection I would have felt better about it.
A better amp seems to wake up the LCD-2s. Music just jumps out at you, specially anything more modern. I can say that my Phoenix, being both powerful and delivering a a wide soundstage gives 'stat-like speed, but with fast and powerful bass and delicious mid-range.