I'm not sure. I think its likely non-harmonic, but that it is correlated to the signal somehow. Probably some kind of inter-modulation distortion. As a physical system, I don't really think it would be properly captured by a signal that seems more suited to testing amps like what I think is going on at Ryu's site.
The funny thing is I don't think I'd hear grain from any of those 'phones on that chart. I've heard the HE-6 and HD800 and I didn't hear any. I've never heard the Lady Gaga but I do have an MTPG which is probably pretty similar but I don't hear any grain from that either. Its as smooth as butter.
Maybe its that "cone break-up" thing that made Senn punch a hole in the middle of the HD800s driver. I think a tiny DD like in an IEM won't have as much of that problem. Its been a while, but IIRC the HD800 probably has the least grain of any full size dynamic I've ever heard.
While we're comparing driver tech, IME BAs do a great job here as well. I haven't heard nearly as many IEMs as I have full size 'phones the few I've heard were grain free as well.